It has been released on DVD:
Quote:
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Originally Posted by https://en.wikipedia.org/wiki/Tarzan_(1966_TV_series)#Home_media
On March 13, 2012, Warner Bros. released Tarzan: Season 1, Part 1 & Tarzan: Season 1, Part 2 on DVD in region 1 via their Warner Archive Collection manufacture-on-demand service.[2][3] The second season was released complete on September 17, 2013.[4]
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Region 1 is North America, so if you live elsewhere (like Australia) you may have trouble playing DVDs from there, depending on how you do that.
Ah, and they’re not expensive:
Amazon has season 1 for about US$25–30 and
season 2 for about US$40. Of course, if you buy them there, there’s the question of how much shipping will cost, not to mention whether they’re willing to mail them to you at all.